- Kevin Spacey as Detective Sergeant Jack "Hollywood Jack" Vincennes
- Russell Crowe as Officer Wendell "Bud" White
- Guy Pearce as Detective Lieutenant Edmund "Shotgun Ed" Exley
- James Cromwell as Captain Dudley Smith
- Kim Basinger as Lynn Bracken
- Danny DeVito as Sid Hudgens
- David Strathairn as Pierce Morehouse Patchett
- Ron Rifkin as District Attorney Ellis Loew
- Graham Beckel as Detective Sergeant Richard "Dick Stens" Stensland
- Amber Smith as Susan Lefferts
- John Mahon as Police Chief
- Paul Guilfoyle as Meyer "Mickey" Cohen
- Matt McCoy as Brett Chase
- Paolo Seganti as Johnny Stompanato
- Simon Baker Denny as Matt Reynolds
- Tomas Arana as Detective Sergeant Michael Breuning
- Michael McCleery as Detective Sergeant William Carlisle
- Shawnee Free Jones as Tammy Jordan
- Darrell Sandeen as Leland "Buzz" Meeks
- Marisol Padilla Sánchez as Inez Soto
- Gwenda Deacon as Mrs. Lefferts
- Jim Metzler as Councilman
- Brenda Bakke as Lana Turner
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